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• W4376128712 abstract "Fluoride-ion batteries (FIBs), which use F– ion migration to drive charge–discharge cycles, have recently gained academic attention as the next generation of rechargeable batteries. Copper difluoride (CuF2) represents a promising positive electrode material for FIBs owing to its high theoretical capacity and high redox potential. In this study, the high-temperature electrochemical reversibility of a CuF2 composite electrode in a bulk-type all-solid-state FIB is evaluated. The CuF2 composite electrode showed high reversible capacities during the initial cycling at operation temperatures as high as 200 °C and relatively good capacity retention up to the 30th cycle, even at 140 °C. It is suggested that the bulk-type battery operates through reversible fluoride-ion shuttling between CuF2 and the counter electrode via an F– ion-conducting solid electrolyte. Furthermore, this study indicates that maintaining a CuF2/Cu particle size of less than 50 nm is important in fabricating bulk-type FIBs with good electrochemical performance." @default.
• W4376128712 created "2023-05-12" @default.
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• W4376128712 date "2023-05-11" @default.
• W4376128712 modified "2023-10-04" @default.
• W4376128712 title "Practical Reversibility of CuF₂ in a Bulk-Type All-Solid-State Fluoride-Ion Battery" @default.
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• W4376128712 doi "https://doi.org/10.1021/acsenergylett.3c00459" @default.
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