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• W4376129835 abstract "A novel Ho3+/Pr3+/Y3+/Gd3+ multiply doped Na5Lu9F32 mixed single crystal was successfully grown via a modified Bridgman technique. The structure of the mixed crystal was characterized by means of X-ray diffraction and Raman spectra. The impacts of Y3+ and Gd3+ ions on the 2.9 μm emission of Na5Lu9F32 single crystals, which incorporated fixed Ho3+/Pr3+, were investigated systematically with the aid of the optical spectra and decay curves of fluorescence. The 2.9 μm emission intensity (Ho3+: 5I6 → 5I7) was further heightened upon gradually introducing both Y3+ and Gd3+ ions into Ho3+/Pr3+-incorporated single crystals pumped at 640 nm. The brokenness of ionic quenching clusters of [Ho3+–Ho3+] and the release of more luminescent ions are in charge of the augment of emission at 2.9 μm by introducing Gd3+ or Y3+ ions into the Ho3+/Pr3+ codoped single crystals. A value of ∼8.2 × 10–21 cm2 was estimated for the maximum emission cross section at 2.9 μm of the mixed crystal. The processing of energy transfer among Ho3+, Pr3+, Y3+, and Gd3+ ions was investigated, and the energy transfer efficiency for Ho3+: 5I7 → Pr3+: 3F2 was approximately 57.32%. The Na5Lu9F32-doped Ho3+/Pr3+/Y3+/Gd3+ mixed crystals may be a new laser gain medium for 2.9 μm generation because of their special spectral and physicochemical properties." @default.
• W4376129835 created "2023-05-12" @default.
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• W4376129835 date "2023-05-11" @default.
• W4376129835 modified "2023-10-15" @default.
• W4376129835 title "Original Na₅(Lu_{1–<i>x</i>–<i>y</i>}Gd_<i>x</i>Y_<i>y</i>)₉F₃₂: Pr³⁺/Ho³⁺ Hybrid Single Crystals for Efficient ∼2.9 μm Mid-Infrared Emission" @default.
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• W4376129835 doi "https://doi.org/10.1021/acs.cgd.3c00383" @default.
• W4376129835 hasPublicationYear "2023" @default.
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