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- W4376132313 abstract "To date, the effect of noble metal (NM) electronic structures on CO2 reaction activity remains unknown, and explicit screening criteria are still lacking for designing highly efficient catalysts in CO2-breathing batteries. Herein, by preferentially considering the decomposition of key intermediate Li2CO3, an intrinsic descriptor constituted of the d x 2 − y 2 ${{rm{d}}}_{{x}^2 - {y}^2}$ orbital states and the electronegativity for predicting high-performance cathode material are discovered. As a demonstration, a series of graphene-supported noble metals ([email protected]) as cathodes are fabricated via a fast laser scribing technique. Consistent with the preliminary prediction, [email protected] exhibits an ultralow overpotential (0.41 V), along with superior cycling performance up to 1400 h. Moreover, the overall thermodynamic reaction pathways on [email protected] confirm the reliability of the established intrinsic descriptor. This basic finding of the relationship between the electronic properties of noble metal cathodes and the performance of Li-CO2 batteries provides a novel avenue for designing remarkably efficient cathode materials for metal-CO2 batteries." @default.
- W4376132313 created "2023-05-12" @default.
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- W4376132313 date "2023-07-02" @default.
- W4376132313 modified "2023-10-16" @default.
- W4376132313 title "Intrinsic Descriptor Guided Noble Metal Cathode Design for Li‐CO<sub>2</sub> Battery" @default.
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- W4376132313 doi "https://doi.org/10.1002/adma.202302325" @default.
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