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• W4376135166 abstract "Magnetophononics, the modulation of magnetic interactions by driving infrared-active lattice excitations, is emerging as a key mechanism for the ultrafast dynamical control of both semiclassical and quantum spin systems by coherent light. We demonstrate that, in a quantum magnet with strong spin-phonon coupling, resonances between the driven phonon and the spin excitation frequencies exhibit an intrinsic self-blocking effect, whereby only a fraction of the available laser power is absorbed by the phonon. Using the quantum master equations governing the nonequilibrium steady states of the coupled spin-lattice system, we show how self-blocking arises from the self-consistent alteration of the resonance frequencies. We link this to the appearance of mutually repelling collective spin-phonon states, which in the regime of strong hybridization become composites of a phonon and two triplons. We then identify the mechanism and optimal phonon frequencies by which to control a global nonequilibrium renormalization of the lattice-driven spin excitation spectrum and demonstrate that this effect should be observable in ultrafast THz experiments on a number of known quantum magnetic materials." @default.
• W4376135166 created "2023-05-12" @default.
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• W4376135166 date "2023-05-11" @default.
• W4376135166 modified "2023-10-17" @default.
• W4376135166 title "Strong-coupling magnetophononics: Self-blocking, phonon-bitriplons, and spin-band engineering" @default.
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• W4376135166 doi "https://doi.org/10.1103/physrevb.107.174415" @default.
• W4376135166 hasPublicationYear "2023" @default.
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