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- W4376138959 abstract "Abstract Electrochemical reduction of CO 2 is an effective method for storing intermittent renewable energy. This could result in fuel additives and chemical feedstocks such as alcohols. A challenge of electrochemical alcohol production is the transfer of electrons and protons, as well as the formation of C–C bonds. As of now, copper-based materials are the most commonly used and effective catalysts. Although CuO x is considered a promising catalyst for electrochemical CO 2 reduction reactions (CO2RR), significant improvements in product selectivity are still needed. This paper presents some results obtained using copper oxide as a cathode, combined with 33% of ionomer, nickel iron as anode, and membrane Fumatech as electrolyte. As a result of physico-chemical experiments, morphological measurements of the cathode, electrochemical experiments carried out with a complete zero-gap cell operating under alkaline conditions, and gas-chromatographic (GC) analyses of the cathode outlet stream, we determined that methyl formate, ethanol, and propanol were mainly obtained at a rate of 116.3 μmol $${text{g}}_{text{cat}}^{-1} , {text{h}}^{-{1}}$$ <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML> <mml:mrow> <mml:msubsup> <mml:mtext>g</mml:mtext> <mml:mrow> <mml:mtext>cat</mml:mtext> </mml:mrow> <mml:mrow> <mml:mo>-</mml:mo> <mml:mn>1</mml:mn> </mml:mrow> </mml:msubsup> <mml:mspace /> <mml:msup> <mml:mrow> <mml:mtext>h</mml:mtext> </mml:mrow> <mml:mrow> <mml:mo>-</mml:mo> <mml:mn>1</mml:mn> </mml:mrow> </mml:msup> </mml:mrow> </mml:math> during operation at 2.2 V." @default.
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- W4376138959 date "2023-05-10" @default.
- W4376138959 modified "2023-10-17" @default.
- W4376138959 title "Alkaline electrolysis using CuOx cathode for the conversion of carbon dioxide into liquid fuels" @default.
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- W4376138959 doi "https://doi.org/10.1007/s40243-023-00235-6" @default.
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