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- W4376270685 abstract "Abstract Nitrogen-containing heterocycles are the key components in many pharmaceuticals and functional materials. In this study, we reported a transition metal-catalyzed high-order reaction sequence for synthesizing a structurally unique N-center 5,6,7-perifused cycle (NCPC). The key characteristics included the formation of a seven-membered ring by the 8π electrocyclization of various alkenes and aromatic heterocycles as π-components, in which metal carbene species generated that further induced the cleavage of the α -C-H or -C-C bond. Specifically, the latter could react with various nucleophilic reagents containing -O, -S, -N, and -C. The stereo-controlled late-stage modification of some complicated pharmaceuticals indicated the versatility of this protocol." @default.
- W4376270685 created "2023-05-13" @default.
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- W4376270685 date "2023-05-12" @default.
- W4376270685 modified "2023-10-16" @default.
- W4376270685 title "Divergently Access N-center 5,6,7-Perifused Cycle" @default.
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- W4376270685 doi "https://doi.org/10.21203/rs.3.rs-2873173/v1" @default.
- W4376270685 hasPublicationYear "2023" @default.
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