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- W4376455764 abstract "The lack of efficient separation membranes limits the development of bio-alcohol purification via a pervaporation process. In this work, novel controllable hydrogen-bonded poly(dimethylsiloxane) (PDMS) membranes are prepared from self-synthesized supramolecular elastomers for alcohol recovery. Different from the conventional covalently-bonded PDMS membranes, the hydrogen-bonding content and therefore the crosslinking degree in the as-synthesized PDMS membranes can be exactly regulated, by the suitable molecular design of the supramolecular elastomers. The effects of hydrogen-bonding content on the flexibility of the polymer chains and the separation performance of the resultant supramolecular membranes are investigated in detail. In comparison with the state-of-the-art polymeric membranes, the novel controllable hydrogen-bonded supramolecular PDMS membrane exhibits ultrahigh fluxes for ethanol (4.1 kg m-2 h-1) and n-butanol (7.7 kg m-2 h-1) recovery from 5 wt% alcohol aqueous solutions at 80 °C, with comparable separation factors. The designed supramolecular elastomer is therefore believed to provide valuable insights into the design of next-generation separation membrane materials for molecular separations." @default.
- W4376455764 created "2023-05-14" @default.
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- W4376455764 date "2023-01-01" @default.
- W4376455764 modified "2023-10-01" @default.
- W4376455764 title "Controllable hydrogen-bonded poly(dimethylsiloxane) (PDMS) membranes for ultrafast alcohol recovery" @default.
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- W4376455764 doi "https://doi.org/10.1039/d3mh00250k" @default.
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