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- W4376503721 abstract "Water adsorption-driven heat transfer (AHT) technology has emerged as a promising solution to address crisis of the global energy consumption and environmental pollution of current heating and cooling processes. Hydrophilicity of water adsorbents plays a decisive role in these applications. This work reports an easy, green, and inexpensive approach to tuning the hydrophilicity of metal-organic frameworks (MOFs) by incorporating mixed linkers, isophthalic acid (IPA), and 3,5-pyridinedicarboxylic acid (PYDC), with various ratios in a series of Al-xIPA-(100-x)PYDC (x: feeding ratio of IPA) MOFs. The designed mixed-linkers MOFs show a variation of hydrophilicity along the fraction of the linkers. Representative compounds with a proportional mixed linker ratio denoted as KMF-2, exhibit an S-shaped isotherm, an excellent coefficient of performance of 0.75 (cooling) and 1.66 (heating) achieved with low driving temperature below 70 °C which offers capability to employ solar or industrial waste heat, remarkable volumetric specific energy capacity (235 kWh m-3 ) and heat-storage capacity (330 kWh m-3 ). The superiority of KMF-2 to IPA or PYDC-containing single-linker MOFs (CAU-10-H and CAU-10pydc, respectively) and most of benchmark adsorbents illustrate the effectiveness of the mixed-linker strategy to design AHT adsorbents with promising performance." @default.
- W4376503721 created "2023-05-15" @default.
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- W4376503721 date "2023-05-13" @default.
- W4376503721 modified "2023-09-25" @default.
- W4376503721 title "Tuning Hydrophilicity of Aluminum MOFs by a Mixed‐Linker Strategy for Enhanced Performance in Water Adsorption‐Driven Heat Allocation Application" @default.
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- W4376503721 doi "https://doi.org/10.1002/advs.202301311" @default.
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