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• W4377013066 abstract "Abstract We report on the development of a Brewster angle-cavity ringdown spectroscopy (BA-CRDS) system for low temperature plasma diagnostics. The system can measure gas species in solutions, with a detection limit (minimum detectable absorbance) of 9.1 × 10 −5 , which is equivalent to a detection limit of 0.04 parts per billion for measuring OH radicals in water at 308 nm. With higher reflectivity ringdown mirrors and improved design of a Brewster angle cell, the detection limit can potentially be up to 10 −6 or lower. In this exploratory study, the absorption cross sections of HgBr 2 and H 2 O 2 in the aqueous phase at 256 nm are measured to be (1.8 ± 0.1) × 10 −18 cm 2 and (5.2 ± 0.5) × 10 −20 cm 2 , respectively. Furthermore, temporal profiles of absorbance from distilled water, HgBr 2 , and H 2 O 2 solutions when interacting with a helium atmospheric plasma jet are individually characterized at different plasma powers, gas flow rates, and/or solute concentrations. The observed linear temporal profiles of absorbance from the plasma-interacted water suggest formation of H 2 O 2 from plasma-generated OH radicals, while the nonlinear temporal profiles from the plasma-treated HgBr 2 solutions reveal possible removal of HgBr 2 by OH radicals. Our results demonstrate that the new BA-CRDS system is a powerful tool for quantification of reactive plasma species in multiphases or other complex settings." @default.
• W4377013066 created "2023-05-19" @default.
• W4377013066 creator A5006999054 @default.
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• W4377013066 date "2023-06-01" @default.
• W4377013066 modified "2023-09-29" @default.
• W4377013066 title "Brewster angle-cavity ringdown spectroscopy for low temperature plasma measurements in multiphases" @default.
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• W4377013066 doi "https://doi.org/10.1088/1361-6595/acd6b6" @default.
• W4377013066 hasPublicationYear "2023" @default.
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