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- W4377013467 abstract "We investigated the dried deposit patterns of quasi-two-dimensional graphene nanoplatelets (GNP) on hydrophilic glass via aqueous sessile droplet evaporation in a saturated alcohol vapor atmosphere. In addition, we studied both the size- and shape-dependent self-assembly and self-sorting of colloids by employing droplets containing bidispersed suspensions comprising GNP and bulk three-dimensional colloidal particles, e.g., polystyrene microspheres (PS). We report distinct self-sorting regimes as the PS diameter Dp varies between 0.1 and 6.4 μm. Under ambient air, the droplet evaporation does not yield discernible self-sorting between GNP and PS. Under saturated alcohol vapor, a critical Dp = 1.1 μm exists, for which the self-sorting does not occur. For Dp < 1.1 μm, the PS sort out from the bidispersed suspension to form the outermost ring of the deposit. The deposit pattern reverses for Dp > 1.1 μm, and GNP deposit on the outermost edge. We corroborate experimental observations with a theoretical model based on the size- and shape-dependent interfacial forces between the colloids." @default.
- W4377013467 created "2023-05-19" @default.
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- W4377013467 date "2023-05-18" @default.
- W4377013467 modified "2023-09-28" @default.
- W4377013467 title "Self-Assembly and Sorting of Graphene Nanoplatelets and Spherical Colloidal Particles via Sessile Droplet Evaporation in Saturated Alcohol Vapor" @default.
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- W4377013467 doi "https://doi.org/10.1021/acs.iecr.3c00796" @default.
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