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• W4377013560 endingPage "26127" @default.
• W4377013560 startingPage "26120" @default.
• W4377013560 abstract "Understanding the deformation of energy storage electrodes at a local scale and its correlation to electrochemical performance is crucial for designing effective electrode architectures. In this work, the effect of electrolyte cation and electrode morphology on birnessite (δ-MnO2) deformation during charge storage in aqueous electrolytes was investigated using a mechanical cyclic voltammetry approach via operando atomic force microscopy (AFM) and molecular dynamics (MD) simulation. In both K2SO4 and Li2SO4 electrolytes, the δ-MnO2 host electrode underwent expansion during cation intercalation, but with different potential dependencies. When intercalating Li+, the δ-MnO2 electrode presents a nonlinear correlation between electrode deformation and electrode height, which is morphologically dependent. These results suggest that the stronger cation-birnessite interaction is the reason for higher local stress heterogeneity when cycling in Li2SO4 electrolyte, which might be the origin of the pronounced electrode degradation in this electrolyte." @default.
• W4377013560 created "2023-05-19" @default.
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• W4377013560 date "2023-05-18" @default.
• W4377013560 modified "2023-10-18" @default.
• W4377013560 title "Effect of Electrode/Electrolyte Coupling on Birnessite (δ-MnO₂) Mechanical Response and Degradation" @default.
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• W4377013560 doi "https://doi.org/10.1021/acsami.3c02055" @default.
• W4377013560 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/37259284" @default.
• W4377013560 hasPublicationYear "2023" @default.
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