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- W4377013954 endingPage "712" @default.
- W4377013954 startingPage "706" @default.
- W4377013954 abstract "Catalytic enantioselective methods that are generally applicable to a broad range of substrates are rare. We report a strategy for the oxidative desymmetrization of meso-diols predicated on a nontraditional catalyst optimization protocol by using a panel of screening substrates rather than a singular model substrate. Critical to this approach was rational modulation of a peptide sequence in the catalyst incorporating a distinct aminoxyl-based active residue. A general catalyst emerged, providing high selectivity in the delivery of enantioenriched lactones across a broad range of diols, while also achieving up to ~100,000 turnovers." @default.
- W4377013954 created "2023-05-19" @default.
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- W4377013954 creator A5073335566 @default.
- W4377013954 date "2023-05-19" @default.
- W4377013954 modified "2023-10-16" @default.
- W4377013954 title "Generality-oriented optimization of enantioselective aminoxyl radical catalysis" @default.
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