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• W4377014001 abstract "Metal halide perovskites are promising for optoelectronic device applications; however, their poor stability under solar illumination remains a primary concern. While the intrinsic photostability of isolated neat perovskite samples has been widely discussed, it is important to explore how charge transport layers─employed in most devices─impact photostability. Herein, we study the effect of organic hole transport layers (HTLs) on light-induced halide segregation and photoluminescence (PL) quenching at perovskite/organic HTL interfaces. By employing a series of organic HTLs, we demonstrate that the HTL’s highest occupied molecular orbital energy dictates behavior; furthermore, we reveal the key role of halogen loss from the perovskite and subsequent permeation into organic HTLs, where it acts as a PL quencher at the interface and introduces additional mass transport pathways to facilitate halide phase separation. In doing so, we both reveal the microscopic mechanism of non-radiative recombination at perovskite/organic HTL interfaces and detail the chemical rationale for closely matching the perovskite/organic HTL energetics to maximize solar cell efficiency and stability." @default.
• W4377014001 created "2023-05-19" @default.
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• W4377014001 date "2023-05-18" @default.
• W4377014001 modified "2023-10-18" @default.
• W4377014001 title "Origins of Photoluminescence Instabilities at Halide Perovskite/Organic Hole Transport Layer Interfaces" @default.
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• W4377014001 doi "https://doi.org/10.1021/jacs.3c03539" @default.
• W4377014001 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/37202123" @default.
• W4377014001 hasPublicationYear "2023" @default.
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