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• W4377019982 abstract "Low-dimensional networked organic-inorganic hybrid metal halide crystal has become an emerging hotspot material due to its opportunities and advantages in the development of white-light-emitting diodes. Therefore, its photoluminescence (PL) mechanism is important. Herein, we study the PL behavior of columniform TPP 2 MnBr 4 crystals using multi-spectroscopy. The temperature-dependent PL data show that the PL of the TPP 2 MnBr 4 crystal originates from the recombination of a self-trapping exciton. A polarization-dependent PL test suggests that the self-trapping exciton is anisotropic, which indicates that the distribution of self-trapping states is sensitive to the orientation of the crystal axis. Space-resolved PL spectroscopy shows that the anisotropy of PL gradually weakens along the orientation of the columniform crystal, which has a longer relaxation distance than traditional light-wave-guiding behavior. Thus, anisotropy of PL can exist before it disappears in the crystal. Our results elucidate the PL mechanism of low-dimensional networked organic-inorganic hybrid metal halide crystals and provide a foundation for advanced optical polarization devices based on them." @default.
• W4377019982 created "2023-05-19" @default.
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• W4377019982 date "2023-06-30" @default.
• W4377019982 modified "2023-10-16" @default.
• W4377019982 title "Optical polarization properties of TPP₂MnBr₄ perovskite crystal adjusted by the self-trapping state" @default.
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• W4377019982 doi "https://doi.org/10.1364/ol.489198" @default.
• W4377019982 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/37450711" @default.
• W4377019982 hasPublicationYear "2023" @default.
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