FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W4377041763> ?p ?o ?g. }

• W4377041763 endingPage "035001" @default.
• W4377041763 startingPage "035001" @default.
• W4377041763 abstract "Abstract We report on the synthesis of LiCrTe <?CDATA $_{textrm{2}}$?> <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML overflow=scroll> <mml:msub> <mml:mi /> <mml:mrow> <mml:mrow> <mml:mtext>2</mml:mtext> </mml:mrow> </mml:mrow> </mml:msub> </mml:math> single crystals and on their anisotropic magnetic properties. We have obtained these single crystals by employing a Te/Li-flux synthesis method. We find LiCrTe <?CDATA $_{textrm{2}}$?> <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML overflow=scroll> <mml:msub> <mml:mi /> <mml:mrow> <mml:mrow> <mml:mtext>2</mml:mtext> </mml:mrow> </mml:mrow> </mml:msub> </mml:math> to crystallize in a TlCdS <?CDATA $_{textrm{2}}$?> <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML overflow=scroll> <mml:msub> <mml:mi /> <mml:mrow> <mml:mrow> <mml:mtext>2</mml:mtext> </mml:mrow> </mml:mrow> </mml:msub> </mml:math> -type structure with cell parameters of a = 3.9512(5) Å and c = 6.6196(7) Å at T = 175 K. The content of lithium in these crystals was determined to be neary stoichiometric by means of neutron diffraction. We find a pronounced magnetic transition at <?CDATA $T^{mathrm{{,}ab}}_{mathrm{N}}$?> <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML overflow=scroll> <mml:msubsup> <mml:mi>T</mml:mi> <mml:mrow> <mml:mrow> <mml:mi mathvariant=normal>N</mml:mi> </mml:mrow> </mml:mrow> <mml:mrow> <mml:mrow> <mml:mrow /> <mml:mi mathvariant=normal>a</mml:mi> <mml:mi mathvariant=normal>b</mml:mi> </mml:mrow> </mml:mrow> </mml:msubsup> </mml:math> = 144 K and <?CDATA $T^{mathrm{{,}c}}_{mathrm{N}}$?> <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML overflow=scroll> <mml:msubsup> <mml:mi>T</mml:mi> <mml:mrow> <mml:mrow> <mml:mi mathvariant=normal>N</mml:mi> </mml:mrow> </mml:mrow> <mml:mrow> <mml:mrow> <mml:mrow /> <mml:mi mathvariant=normal>c</mml:mi> </mml:mrow> </mml:mrow> </mml:msubsup> </mml:math> = 148 K, respectively. These transition temperatures are substantially higher than earlier reports on polycrystalline samples. We have performed neutron powder diffraction measurements that reveal that the long-range low-temperature magnetic structure of single crystalline LiCrTe <?CDATA $_{textrm{2}}$?> <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML overflow=scroll> <mml:msub> <mml:mi /> <mml:mrow> <mml:mrow> <mml:mtext>2</mml:mtext> </mml:mrow> </mml:mrow> </mml:msub> </mml:math> is an A-type antiferromagnetic structure. Our DFT calculations are in good agreement with these experimental observations. We find the system to be easy axis with moments oriented along the c -direction experimentally as well as in our calculations. Thereby, the magnetic Hamiltonian can be written as <?CDATA $H = H_{mathrm{Heisenberg}} + sum_i K_c (S_i^z)^2$?> <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML overflow=scroll> <mml:mi>H</mml:mi> <mml:mo>=</mml:mo> <mml:msub> <mml:mi>H</mml:mi> <mml:mrow> <mml:mrow> <mml:mi mathvariant=normal>H</mml:mi> <mml:mi mathvariant=normal>e</mml:mi> <mml:mi mathvariant=normal>i</mml:mi> <mml:mi mathvariant=normal>s</mml:mi> <mml:mi mathvariant=normal>e</mml:mi> <mml:mi mathvariant=normal>n</mml:mi> <mml:mi mathvariant=normal>b</mml:mi> <mml:mi mathvariant=normal>e</mml:mi> <mml:mi mathvariant=normal>r</mml:mi> <mml:mi mathvariant=normal>g</mml:mi> </mml:mrow> </mml:mrow> </mml:msub> <mml:mo>+</mml:mo> <mml:mrow> <mml:munder> <mml:mo>∑</mml:mo> <mml:mi>i</mml:mi> </mml:munder> </mml:mrow> <mml:msub> <mml:mi>K</mml:mi> <mml:mi>c</mml:mi> </mml:msub> <mml:mo stretchy=false>(</mml:mo> <mml:msubsup> <mml:mi>S</mml:mi> <mml:mi>i</mml:mi> <mml:mi>z</mml:mi> </mml:msubsup> <mml:mrow> <mml:msup> <mml:mo stretchy=false>)</mml:mo> <mml:mn>2</mml:mn> </mml:msup> </mml:mrow> </mml:math> with <?CDATA $K_c = -0.34$?> <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML overflow=scroll> <mml:msub> <mml:mi>K</mml:mi> <mml:mi>c</mml:mi> </mml:msub> <mml:mo>=</mml:mo> <mml:mo>−</mml:mo> <mml:mn>0.34</mml:mn> </mml:math> K (where <?CDATA $|S^z| = frac{3}{2}$?> <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML overflow=scroll> <mml:mrow> <mml:mo>|</mml:mo> </mml:mrow> <mml:msup> <mml:mi>S</mml:mi> <mml:mi>z</mml:mi> </mml:msup> <mml:mrow> <mml:mo>|</mml:mo> </mml:mrow> <mml:mo>=</mml:mo> <mml:mfrac> <mml:mn>3</mml:mn> <mml:mn>2</mml:mn> </mml:mfrac> </mml:math> ). We find LiCrTe <?CDATA $_{textrm{2}}$?> <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML overflow=scroll> <mml:msub> <mml:mi /> <mml:mrow> <mml:mrow> <mml:mtext>2</mml:mtext> </mml:mrow> </mml:mrow> </mml:msub> </mml:math> to be highly anisotropic, with a pronounced metamagnetic transition for <?CDATA $H perp ab$?> <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML overflow=scroll> <mml:mi>H</mml:mi> <mml:mo>⊥</mml:mo> <mml:mi>a</mml:mi> <mml:mi>b</mml:mi> </mml:math> with a critical field of <?CDATA $mu H_{MM}$?> <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML overflow=scroll> <mml:mi>μ</mml:mi> <mml:msub> <mml:mi>H</mml:mi> <mml:mrow> <mml:mi>M</mml:mi> <mml:mi>M</mml:mi> </mml:mrow> </mml:msub> </mml:math> (5 K) ≈ 2.5 T. Using detailed orientation-dependent magnetization measurements, we have determined the magnetic phase diagram of this material. Our findings suggest that LiCrTe <?CDATA $_{textrm{2}}$?> <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML overflow=scroll> <mml:msub> <mml:mi /> <mml:mrow> <mml:mrow> <mml:mtext>2</mml:mtext> </mml:mrow> </mml:mrow> </mml:msub> </mml:math> is a promising material for exploring the interplay between crystal structure and magnetism, and could have potential applications in spin-based 2D devices." @default.
• W4377041763 created "2023-05-19" @default.
• W4377041763 creator A5013458803 @default.
• W4377041763 creator A5020865701 @default.
• W4377041763 creator A5028120302 @default.
• W4377041763 creator A5029481648 @default.
• W4377041763 creator A5035163984 @default.
• W4377041763 creator A5055095051 @default.
• W4377041763 creator A5062397531 @default.
• W4377041763 date "2023-05-17" @default.
• W4377041763 modified "2023-10-01" @default.
• W4377041763 title "Synthesis and anisotropic magnetic properties of LiCrTe 2 single crystals with a triangular-lattice antiferromagnetic structure" @default.
• W4377041763 cites W1969274491 @default.
• W4377041763 cites W1974378834 @default.
• W4377041763 cites W1981368803 @default.
• W4377041763 cites W1996473407 @default.
• W4377041763 cites W1998981899 @default.
• W4377041763 cites W2020363296 @default.
• W4377041763 cites W2023003113 @default.
• W4377041763 cites W2030117421 @default.
• W4377041763 cites W2031392878 @default.
• W4377041763 cites W2039972361 @default.
• W4377041763 cites W2061660128 @default.
• W4377041763 cites W2069836644 @default.
• W4377041763 cites W2070835228 @default.
• W4377041763 cites W2080400224 @default.
• W4377041763 cites W2086128308 @default.
• W4377041763 cites W2094603083 @default.
• W4377041763 cites W2103279820 @default.
• W4377041763 cites W2148514557 @default.
• W4377041763 cites W2157058142 @default.
• W4377041763 cites W2227891475 @default.
• W4377041763 cites W2330279691 @default.
• W4377041763 cites W2470768772 @default.
• W4377041763 cites W2473326270 @default.
• W4377041763 cites W248076057 @default.
• W4377041763 cites W2606397457 @default.
• W4377041763 cites W2752885377 @default.
• W4377041763 cites W2794348381 @default.
• W4377041763 cites W2939236527 @default.
• W4377041763 cites W2941211088 @default.
• W4377041763 cites W2953243305 @default.
• W4377041763 cites W2971731529 @default.
• W4377041763 cites W2994753016 @default.
• W4377041763 cites W3024523300 @default.
• W4377041763 cites W3082117128 @default.
• W4377041763 cites W3098634202 @default.
• W4377041763 cites W3100446431 @default.
• W4377041763 cites W3206776128 @default.
• W4377041763 cites W3208299838 @default.
• W4377041763 cites W4213272049 @default.
• W4377041763 cites W4290878972 @default.
• W4377041763 cites W4311766812 @default.
• W4377041763 doi "https://doi.org/10.1088/2515-7639/acd27a" @default.
• W4377041763 hasPublicationYear "2023" @default.
• W4377041763 type Work @default.
• W4377041763 citedByCount "0" @default.
• W4377041763 crossrefType "journal-article" @default.
• W4377041763 hasAuthorship W4377041763A5013458803 @default.
• W4377041763 hasAuthorship W4377041763A5020865701 @default.
• W4377041763 hasAuthorship W4377041763A5028120302 @default.
• W4377041763 hasAuthorship W4377041763A5029481648 @default.
• W4377041763 hasAuthorship W4377041763A5035163984 @default.
• W4377041763 hasAuthorship W4377041763A5055095051 @default.
• W4377041763 hasAuthorship W4377041763A5062397531 @default.
• W4377041763 hasBestOaLocation W43770417631 @default.
• W4377041763 hasConcept C11413529 @default.
• W4377041763 hasConcept C192562407 @default.
• W4377041763 hasConcept C41008148 @default.
• W4377041763 hasConceptScore W4377041763C11413529 @default.
• W4377041763 hasConceptScore W4377041763C192562407 @default.
• W4377041763 hasConceptScore W4377041763C41008148 @default.
• W4377041763 hasFunder F4320320924 @default.
• W4377041763 hasFunder F4320322581 @default.
• W4377041763 hasFunder F4320327257 @default.
• W4377041763 hasIssue "3" @default.
• W4377041763 hasLocation W43770417631 @default.
• W4377041763 hasOpenAccess W4377041763 @default.
• W4377041763 hasPrimaryLocation W43770417631 @default.
• W4377041763 hasRelatedWork W2018879842 @default.
• W4377041763 hasRelatedWork W2040490366 @default.
• W4377041763 hasRelatedWork W2325423348 @default.
• W4377041763 hasRelatedWork W2737498735 @default.
• W4377041763 hasRelatedWork W2744391499 @default.
• W4377041763 hasRelatedWork W2898370298 @default.
• W4377041763 hasRelatedWork W2899084033 @default.
• W4377041763 hasRelatedWork W3120461830 @default.
• W4377041763 hasRelatedWork W3144504424 @default.
• W4377041763 hasRelatedWork W4292492973 @default.
• W4377041763 hasVolume "6" @default.
• W4377041763 isParatext "false" @default.
• W4377041763 isRetracted "false" @default.
• W4377041763 workType "article" @default.