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- W4377693352 abstract "Lithium-rich layered oxides (LRLOs), with the chemical formula of xLi2MnO3·(1 – x)LiMO2, delivering higher specific discharge capacity, are potential cathode materials for lithium-ion batteries. However, the dissolution of transition metal ions and the instability of the cathode-electrolyte interphase (CEI) hinder the commercial application of LRLOs. Herein, a simple and affordable method is developed for the construction of a robust CEI layer by quenching a kind of cobalt-free LRLO, Li1.2Ni0.15Fe0.1Mn0.55O2 (denoted as NFM), in 1,1,2,2-tetrafluoroethyl-2,2,2-trifluoroethyl ether solvent. This robust CEI, with well-distributed LiF, TMFx, and partial organic component CFx, performs as a physical barrier to prevent NFM from direct contact with the electrolyte, suppresses the oxygen release, and ensures the CEI layer stability. The customized CEI with LiF and TMFx-rich phase considerably enhances the NFM cycle stability and the initial coulomb efficiency and inhibits voltage fading. This work provides a valuable strategy for designing stable interface chemistry on the cathode of lithium-ion batteries." @default.
- W4377693352 created "2023-05-24" @default.
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- W4377693352 date "2023-05-23" @default.
- W4377693352 modified "2023-09-27" @default.
- W4377693352 title "Construction of Inorganic-Rich Cathode Electrolyte Interphase on Co-Free Cathodes" @default.
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- W4377693352 doi "https://doi.org/10.1021/acsami.3c02553" @default.
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