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- W4377990580 abstract "The non-aqueous redox flow battery (NARFB) is a very promising technology for the grid-scale energy storage; however, its wide application is seriously limited by the cycling stability. Here, we designed a ferrocene derivative by imidazole-functionalization and grafting an oligoether chain, 1-ferrocenylmethyl-3-(2-(2-(2-methoxyethoxy)ethoxy)ethyl) imidazolium-bis(trifluoromethylsulfonyl)imide (FcMITEGTFSI). The imidazolium cationic group induces a positive shift in the redox potential of the ferrocene core whilst ensuring the stability of the active species; the flexible oligoether side chain renders the molecule a liquid at room temperature (25 °C) and miscible with acetonitrile solvent. The flow battery shows robust cycling stability, with an overall discharge capacity retention of ≈95.5% after 200 cycles, corresponding to a capacity retention of ≈99.98% per cycle at 25 mA cm−2 with 0.1 M electrolyte." @default.
- W4377990580 created "2023-05-25" @default.
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- W4377990580 creator A5056989890 @default.
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- W4377990580 date "2023-07-01" @default.
- W4377990580 modified "2023-09-24" @default.
- W4377990580 title "Imidazolium-functionalized liquid ferrocene derivative positive material enables robust cycling stability of non-aqueous redox flow battery" @default.
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- W4377990580 doi "https://doi.org/10.1016/j.cej.2023.143697" @default.
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