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- W4378348495 abstract "Zn dendrite growth and undesired parasitic reactions severely restrict the practical use of deep-cycling Zn metal anodes (ZMAs). Herein, we demonstrate an elaborate design of atomically dispersed Cu and Zn sites anchored on N,P-codoped carbon macroporous fibers (denoted as Cu/Zn-N/P-CMFs) as a three-dimensional (3D) versatile host for efficient ZMAs in mildly acidic electrolyte. The 3D macroporous frameworks can alleviate the structural stress and suppress Zn dendrite growth by spatially homogenizing Zn2+ flux. Moreover, the well-dispersed Cu and Zn atoms anchored by N and P atoms maximize the utilization as abundant active nucleation sites for Zn plating. As expected, the Cu/Zn-N/P-CMFs host presents a low Zn nucleation overpotential, high reversibility, and dendrite-free Zn deposition. The Cu/Zn-N/P-CMFs-Zn electrode exhibits stable Zn plating/stripping with low polarization for 630 h at 2 mA cm–2 and 2 mAh cm–2. When coupled with a MnO2 cathode, the fabricated full cell also shows impressive cycling performance even when tested under harsh conditions." @default.
- W4378348495 created "2023-05-27" @default.
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- W4378348495 date "2023-05-26" @default.
- W4378348495 modified "2023-10-14" @default.
- W4378348495 title "Atomically Dispersed Zincophilic Sites in N,P-Codoped Carbon Macroporous Fibers Enable Efficient Zn Metal Anodes" @default.
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- W4378348495 doi "https://doi.org/10.1021/jacs.3c03030" @default.
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