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• W4378363578 endingPage "758" @default.
• W4378363578 startingPage "727" @default.
• W4378363578 abstract "Efficient and mild cleavage of CC bonds has a significant synthetic potential. There is a demand for practical methods for breaking CC bonds starting from a variety of substrates where the original functional groups serve as temporary activating or directing group in a number of synthetic processes. In this chapter an overview of the most recent and widely applicable dehomologation methodologies is provided. The chapter has been organized based on the functional group of the starting material, in detail carboxylic acids and derivatives, alcohols, carbohydrates, aldehydes, and derivatives. A short final section is dedicated to miscellaneous dehomologation reactions, which cannot be classified in the previous classes. The proposed strategies range from the use of oxidants as hypervalent iodine to transition metals and photoredox catalysis. New functional groups are thus accessible to design subsequent post-modification applications. Taken together, the proposed dehomologation strategies form the basis for the fragmentation of important structural motifs obtained from complex organic molecules and represent a toolkit for transformative processes applicable to biomass conversion." @default.
• W4378363578 created "2023-05-27" @default.
• W4378363578 creator A5064531741 @default.
• W4378363578 creator A5087144458 @default.
• W4378363578 date "2023-05-26" @default.
• W4378363578 modified "2023-09-25" @default.
• W4378363578 title "Dehomologations: Ring Contractions" @default.
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