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• W4378602904 abstract "Oxides are emerging candidates for mid-infrared (mid-IR) nonlinear optical (NLO) materials. However, their intrinsically weak second harmonic generation (SHG) effects hinder their further development. A major design challenge is to increase the nonlinear coefficient while maintaining the broad mid-IR transmission and high laser-induced damage threshold (LIDT) of the oxides. In this study, it is reported on a polar NLO tellurite, Cd2 Nb2 Te4 O15 (CNTO), featuring a pseudo-Aurivillius-type perovskite layered structure composed of three types of NLO active groups, including CdO6 octahedra, NbO6 octahedra, and TeO4 seesaws. The uniform orientation of the distorted units induces a giant SHG response that is ≈31 times larger than that of KH2 PO4 , the largest value among all reported metal tellurites. Additionally, CNTO exhibits a large band gap (3.75 eV), a wide optical transparency window (0.33-14.5 µm), superior birefringence (0.12@ 546 nm), high LIDT (23 × AgGaS2 ), and strong acid and alkali resistance, indicating its potential as a promising mid-IR NLO material." @default.
• W4378602904 created "2023-05-29" @default.
• W4378602904 creator A5000025780 @default.
• W4378602904 creator A5015534012 @default.
• W4378602904 creator A5020527447 @default.
• W4378602904 creator A5030863883 @default.
• W4378602904 creator A5038113064 @default.
• W4378602904 creator A5054799694 @default.
• W4378602904 date "2023-05-28" @default.
• W4378602904 modified "2023-10-14" @default.
• W4378602904 title "Cd₂Nb₂Te₄O₁₅: A Novel Pseudo‐Aurivillius‐Type Tellurite with Unprecedented Nonlinear Optical Properties and Excellent Stability" @default.
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