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- W4378781623 abstract "The artificial olfaction units (or e-noses) capable of room-temperature operation are highly demanded to meet the requests of society in numerous vital applications and developing Internet-of-Things. Derivatized 2D crystals are considered as sensing elements of choice in this regard, unlocking the potential of the advanced e-nose technologies limited by the current semiconductor technologies. Herein, we consider fabrication and gas-sensing properties of On-chip multisensor arrays based on a hole-matrixed carbonylated (C-ny) graphene film with a gradually changed thickness and concentration of ketone groups of up to 12.5 at.%. The enhanced chemiresistive response of C-ny graphene toward methanol and ethanol, of hundred ppm concentration when mixing with air to match permissible exposure OSHA limits, at room-temperature operation is signified. Following thorough characterization via core-level techniques and density functional theory, the predominant role of the C-ny graphene-perforated structure and abundance of ketone groups in advancing the chemiresistive effect is established. Advancing practice applications, selective discrimination of the studied alcohols is approached by linear discriminant analysis employing a multisensor array’s vector signal, and the fabricated chip’s long-term performance is shown." @default.
- W4378781623 created "2023-06-01" @default.
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- W4378781623 date "2023-05-30" @default.
- W4378781623 modified "2023-10-11" @default.
- W4378781623 title "Toward On-Chip Multisensor Arrays for Selective Methanol and Ethanol Detection at Room Temperature: Capitalizing the Graphene Carbonylation" @default.
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- W4378781623 doi "https://doi.org/10.1021/acsami.3c02833" @default.
- W4378781623 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/37253093" @default.
- W4378781623 hasPublicationYear "2023" @default.
- W4378781623 type Work @default.