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- W4378840265 abstract "Inorganic cesium lead bromide (CsPbBr3) perovskite nanocrystals (PNCs) have shown promise in optoelectronic applications. A simpler method of synthesizing high-quality PNCs is the ligand-assisted reprecipitation (LARP) method, but it is susceptible to instability. This study used a high-throughput automated experimental platform to explore the growth behaviors and colloidal stability of LARP-synthesized PNCs. The influence of ligands on particle growth and functionalities was systematically explored using two distinctive acid-base pairs. The study found that short-chain ligands cannot make functional PNCs with the desired sizes and shapes, whereas long-chain ligands provide homogeneous and stable PNCs. The study also found that excessive amines or polar antisolvents can cause PNCs to transform into a Cs-rich non-perovskite structure with poorer emission functionalities and larger size distributions. The diffusion of ligands in a reaction system is crucial in determining the structures and functionalities of the PNCs. This study provides detailed guidance on synthesis routes for desired PNCs." @default.
- W4378840265 created "2023-06-01" @default.
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- W4378840265 date "2023-09-01" @default.
- W4378840265 modified "2023-10-14" @default.
- W4378840265 title "Understanding the ligand-assisted reprecipitation of CsPbBr3 nanocrystals via high-throughput robotic synthesis approach" @default.
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- W4378840265 doi "https://doi.org/10.1016/j.matt.2023.05.023" @default.
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