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• W4379209764 endingPage "108644" @default.
• W4379209764 startingPage "108644" @default.
• W4379209764 abstract "The construction of hydrogels with good mechanical properties and phosphorescent properties is full of challenges. Herein, we report a supramolecular phosphorescent hydrogel with long lifetime, high tensile strength and self-healing property, which can be easily constructed through in-situ thermal-initiated polymerization of isocyanatoethyl acrylate-modified β-cyclodextrin (β-CD-DA) and acrylate-modified adamantane (Ad-DA), acrylic acid (AA), followed by the non-covalent association with carbon dots (CNDs). The lifetime of phosphorescent hydrogel can reach 1261 ms at room temperature, and the quantum yield is 11%. Importantly, through the efficient triplet to singlet Förster resonance energy transfer (TS-FRET), the phosphorescent hydrogel shows the good phosphorescence energy transfer property for organic dyes Rhodamine B and Eosin Y with the delayed fluorescence lifetime up to 730 ms and 585 ms as well as the energy transfer efficiency (ΦET) up to 99.9% and 99.3%, respectively. Moreover, owing to the host-guest interactions between β-CD-DA and Ad-DA, the three-dimensional cross-linked network phosphorescent hydrogel can be easily stretched to 18 times of its original length, and can achieve self-healing of the cut surfaces within 30 minutes. These results will expand the scope of phosphorescent materials and provide new ideas and opportunities for materials science." @default.
• W4379209764 created "2023-06-04" @default.
• W4379209764 creator A5054726579 @default.
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• W4379209764 date "2023-06-01" @default.
• W4379209764 modified "2023-10-12" @default.
• W4379209764 title "In situ crosslink polymerization induced long-lived multicolor supramolecular hydrogel based on modified β-cyclodextrin" @default.
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• W4379209764 doi "https://doi.org/10.1016/j.cclet.2023.108644" @default.
• W4379209764 hasPublicationYear "2023" @default.
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