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- W4379535636 abstract "Abstract. Nucleophilic high-molecular-weight organic compounds (HMWOC) are sensitive to proton (H+) in FT-ICR MS analysis. A comprehensive evaluation of diurnal evolution of nucleophilic HMWOC was performed. HMWOCs aged significantly in daily cycles, accompanied by functionality shifts, particularly oxygenated and reduced nitrogen (CHON and CHN) and oxygenated organics. The intensities of HMW oxygenated compounds increased during daytime and nighttime. The daytime evolution produced more nitrogen-containing compounds with carboxylic groups (–COOH) homologs with molecular weights greater than 300, while the nighttime evolution produced mostly small CHON compounds (molecular weights <300). During evolution, nighttime CHON removals were also observed; meanwhile, carboxylation was also identified in CHON groups. The daytime evolution produced significantly more reduced nitrogen-containing compounds and a day- and nighttime increase in CHN compounds with five members was also observed. This study can provide insights into the aging of less polar organic aerosols." @default.
- W4379535636 created "2023-06-07" @default.
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- W4379535636 date "2023-06-06" @default.
- W4379535636 modified "2023-10-10" @default.
- W4379535636 title "Evolution of Nucleophilic High-molecular-weight Organic Compounds in Ambient Aerosols" @default.
- W4379535636 doi "https://doi.org/10.5194/egusphere-2023-936" @default.
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