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- W4379741903 endingPage "143943" @default.
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- W4379741903 abstract "In this study, we have successfully prepared a freeze-resistant conductive hydrogel with a fast polymerization rate and excellent mechanical and adhesive properties. In this paper, hydrogels capable of rapid polymerization in a short time were prepared based on the [email protected] (WSCA, water-soluble cellulose acetate; [email protected], tannic acid-coated WSCA suspension; [email protected], a certain amount of zinc chloride (ZnCl2) was added to [email protected] suspension;) autocatalytic system at room temperature or low temperature. [email protected] forms a stable reversible quinone-catechol redox reaction to activate the decomposition of ammonium persulfate (APS, initiator) to produce SO4−· radicals, which triggers the ultra-fast polymerization of amphoteric ([2-(methacryloyloxy) ethyl] dimethyl-(3-sulfopropyl), SBMA) and acrylic monomers (AA). To improve the frost resistance and electrical conductivity of the hydrogels, we also introduced amphoteric ions, which can provide migration channels for Zn2+ and greatly increase the migration rate. The [email protected]/PSA hydrogel (PSA, hydrogel prepared by polymerization of acrylic acid and SBMA as monomers;) can achieve tensile strength and toughness of 1.33 MPa and 4.89 MJ m−3. It can provide excellent electrical conductivity and interfacial adhesion over a temperature range of 25 to −60 °C. In addition, the supercapacitor assembled from the [email protected]/PSA hydrogel electrolyte still has good capacitance characteristics after folding and 10,000 charge/discharge cycles, with a capacitance retention of 93.33 % and an excellent cycle life. This autocatalytic system provides a new strategy and approach for the preparation of freeze-resistant conductive hydrogel electrolytes." @default.
- W4379741903 created "2023-06-08" @default.
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- W4379741903 date "2023-08-01" @default.
- W4379741903 modified "2023-10-16" @default.
- W4379741903 title "Self-adhesive frost-resistant conductive hydrogel electrolytes based on TA@WSCA-Zn autocatalytic system for flexible and foldable solid-state capacitors" @default.
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- W4379741903 doi "https://doi.org/10.1016/j.cej.2023.143943" @default.
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