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• W4379931919 abstract "Novel tri-N-heterocyclic carbene (triNHC)-coordinated iridium catalysts (Ir(triNHC)) were employed for generating clean hydrogen and useful Cn acids from biomass-derived alcohols. The high efficiency and fast rate of hydrogen production (maximum turnover frequency = 13,080 h–1 and 485 L of H2/g-cat·h) from sustainable ethylene glycol were elucidated by the increased electron-richness of Ir(triNHC) complexes where three NHC ligands were coordinated to an iridium(I) ion. Elaborated mechanistic studies support the proposed reaction mechanisms forming H2 and Cn acids. This Ir(triNHC)-catalyzed process converting sustainable alcohols to useful fuels and chemicals is a promising carbon-neutral process." @default.
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• W4379931919 date "2023-06-08" @default.
• W4379931919 modified "2023-10-18" @default.
• W4379931919 title "Ir(tri-<i>N</i>-Heterocyclic Carbene)-Catalyzed Production of Hydrogen and C_<i>n</i> Acids from Ethylene Glycol" @default.
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• W4379931919 doi "https://doi.org/10.1021/acssuschemeng.3c00950" @default.
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