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- W4379980694 abstract "Abstract Novel alginate-based binders containing either catechol (d-Alg) or sulfonate (s-Alg) functional groups were developed and characterized to improve the capacity decay performance and better stability of Li-ion batteries. The electrochemical performance of silicon-graphite (Si/Gr) anode with alginate-based binder was compared to the commonly used CMC/SBR binder. The active material in the anodes was the ball-milled Si/Gr (20:80 wt%) powder mixture. A comprehensive electrochemical study was carried out through rate capability test, cycle test, differential capacity analysis (d Q /d V ), and electrochemical impedance spectroscopy (EIS). The functionalized s-Alg binder showed the lowest electrolyte uptake (11.5%) and the highest tensile strength (97 MPa). Anodes with s-Alg exhibited high initial capacity (1250 mAh g − 1 ) and improved decay performance (580 mAh g − 1 at 0.2 C), by ~ 65% higher compared to CMC/SBR binder. The influence of pH value of s-Alg binder preparation showed that anodes prepared at pH 3 of s-Alg exhibit better performance, reaching 800 and 750 mAh g − 1 at 0.1 C and 0.2 C, respectively due to the stronger bonding formation and compactness of anode layer which providing low charge transfer and solid electrolyte interface resistance." @default.
- W4379980694 created "2023-06-10" @default.
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- W4379980694 date "2023-06-09" @default.
- W4379980694 modified "2023-10-11" @default.
- W4379980694 title "Novel alginate-based binders for silicon-graphite anodes in lithium-ion batteries: Effect of binder chemistry on the electrochemical performance" @default.
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- W4379980694 doi "https://doi.org/10.21203/rs.3.rs-3033169/v1" @default.
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