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- W4380051570 abstract "Abstract Radicals can be formed expeditiously through the direct irradiation of an electron donor‐acceptor (EDA) complex. Herein, we show a photocatalyst‐free strategy for gem ‐difluoroalkenes synthesis realized by photo‐irradiation of the EDA complexes, which can be generated in situ between N ‐alkylpyridinium salts and Hantzsch ester without any other additives. A wide variety of readily available alkylamines underwent deaminative defluoroalkylation to provide the corresponding gem ‐difluoroalkenes. This reaction system exhibits high reactivity and good functional group tolerance and provides a practical and effective entry to a broad range of α ‐alkyl‐substituted gem ‐difluoroalkenes." @default.
- W4380051570 created "2023-06-10" @default.
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- W4380051570 date "2023-06-06" @default.
- W4380051570 modified "2023-10-15" @default.
- W4380051570 title "Catalyst‐Free Defluoroalkylation of Trifluoromethylated Alkenes via Photoinduced Electron Donor‐Acceptor Complex" @default.
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- W4380051570 doi "https://doi.org/10.1002/slct.202300665" @default.
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