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- W4380078741 abstract "A Zr-catalyzed synthesis of tetrasubstituted 1,3-diacylpyrroles is reported that employs the direct use of N-acyl α-aminoaldehydes with 1,3-dicarbonyl compounds. The products were formed in up to 88% yield and shown to be hydrolytically and configurationally stable under the reaction conditions (THF/1,4-dioxane and H2O). The N-acyl α-aminoaldehydes were readily prepared from the corresponding α-amino acids. The reaction tolerates a wide array of substrate types including alkyl-, aryl-, heteroaryl-, and heteroatom-containing groups on the aminoaldehyde side chain. A variety of 1,3-dicarbonyls proved amenable to the reaction along with an aldehyde derived from a l,l-dipeptide, an aldehyde generated in situ, and an N-acylated glucosamine." @default.
- W4380078741 created "2023-06-10" @default.
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- W4380078741 date "2023-06-09" @default.
- W4380078741 modified "2023-09-25" @default.
- W4380078741 title "Zr-Catalyzed Synthesis of Tetrasubstituted 1,3-Diacylpyrroles from <i>N</i>-Acyl α-Aminoaldehydes and 1,3-Dicarbonyls" @default.
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- W4380078741 doi "https://doi.org/10.1021/acs.joc.3c00675" @default.
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