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- W4380201458 abstract "The single atom solution is proposed for the CO2 methanation. The catalytic mechanism of single atom solution on the methanation of CO2 is studied. The catalytic performance of single atom solution with different solution proportions was experimentally determined. It was found that each gram of metal atom afforded to produce 294.50 g of methane and 9.24 g of hydrogen. The stability of catalytic performance and good cycling performance of the CO2 conversion reaction were verified. A DFT model was developed to analyze the microscopic mechanism of CO2 methanation by single atom solution. It was found that the reaction path formed by COOH* intermediates is the more easily realized reaction path. It is calculated that the conversion of CO* to HCO* was the rate-limiting step of the optimal reaction path, which corresponded to a limiting potential of 0.85 V. The conversion of CO2 by single atom solution provides a new direction." @default.
- W4380201458 created "2023-06-11" @default.
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- W4380201458 date "2023-11-01" @default.
- W4380201458 modified "2023-10-03" @default.
- W4380201458 title "Experimental and DFT study on single atom solution for carbon dioxide methanation" @default.
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- W4380201458 doi "https://doi.org/10.1016/j.fuel.2023.128911" @default.
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