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- W4380302854 abstract "Bulk copolymerization of alkyl acrylate and cyclodextrin (CD) host monomers forms a single movable cross network (SC), in which the CD units act as movable cross-linkers. Moreover, the bulk copolymerization of the CD monomer and main chain monomer in the presence of SC results in dual-cross-network (DC) elastomers. DC elastomers result in good toughness (Gf). Here, to improve Gf and Young’s modulus (E), we hybridized DC elastomers with tertiary glassy polymers, which are called DCP elastomers. We prepared the DCP elastomers by photopolymerization of N,N-dimethylacrylamide (DMAA) and poly(2-methoxyethyl acrylate) (MEA) in the presence of DC. A DCP elastomer with a suitable weight percent (wt %) of the glassy polymer shows high Gf (108.4 MJ m–3) and E (223.4 MPa) values. Dynamic mechanical analysis (DMA) and in situ small-angle X-ray scattering (SAXS) measurements under uniaxial stretching indicate multiple deformations based on phase-separated structures. We suggest that the phase-separated structures of DCP elastomers cause a large stress dissipation, which contributes to high toughness." @default.
- W4380302854 created "2023-06-13" @default.
- W4380302854 creator A5004246153 @default.
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- W4380302854 date "2023-06-12" @default.
- W4380302854 modified "2023-10-17" @default.
- W4380302854 title "Hybridizing a Dual-Cross Network and a Linear Glassy Polymer for Dynamic Contributions to High Mechanical Toughness Based on Phase-Separated Structures" @default.
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- W4380302854 doi "https://doi.org/10.1021/acs.macromol.3c00178" @default.
- W4380302854 hasPublicationYear "2023" @default.
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