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- W4380422483 abstract "Several dumbbell conjugates featuring M3N@Ih-C80 (M = Sc, Y) and C60 were prepared to systematically investigate interfullerene electronic interactions and excited state dynamics. From electrochemical investigations, we concluded that the redox potentials of our M3N@Ih-C80 (M = Sc, Y) dumbbells depend largely on the interfullerene electronic interactions. Assisted by DFT calculation, the unique role of metal atoms was highlighted. Most importantly, ultrafast spectroscopy experiments revealed symmetry-breaking charge separation in Sc3N@C80-dumbbell to yield an unprecedented (Sc3N@C80)•+-(Sc3N@C80)•– charge separated state. This is, to the best of our knowledge, the first time that symmetry-breaking charge separation following photoexcitation is corroborated in a fullerene system. As such, our work shed light on the significance of interfullerene electronic interactions and their uniqueness for modulating excited state properties." @default.
- W4380422483 created "2023-06-14" @default.
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- W4380422483 date "2023-06-13" @default.
- W4380422483 modified "2023-10-17" @default.
- W4380422483 title "Interfullerene Electronic Interactions and Excited-State Dynamics in Fullerene Dumbbell Conjugates" @default.
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- W4380422483 doi "https://doi.org/10.1021/jacs.3c03486" @default.
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