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- W4380489021 abstract "Polylactide (PLA) is regarded as one of the most promising substitutes for petroleum-based thermoplastics, but the inherent nature of hydrophilicity and poor toughness severely limits its widespread application. In this work, PLA films with superhydrophobicity and outstanding mechanical properties are fabricated by combing “annealing stretching” and nonsolvent-induced phase separation (NIPS)-based surface modification. The prepared films have low surface adhesion characteristics, exhibiting water contact angles of up to 163.4° and extremely small sliding angles as low as 1°. Excellent self-cleaning function to solid contaminates and good repellency to several liquid contaminates are also demonstrated. In addition, the strong interfacial adhesion between the structured surface coating and the substrate enables the PLA films to resist various chemical and mechanical damages, exhibiting splendid durability under severe environmental conditions. Moreover, a superb stiffness–toughness balance is obtained. The tensile strength, Young’s modulus, and elongation at break of the fabricated PLA film are 98.9 MPa, 2.87 GPa, and 91.7%, respectively, which are dramatically improved compared to that of the unstructured casting PLA film (57.6 MPa, 1.57 GPa, and 21.0%, respectively). This work would provide significant guidance for the facile and potentially large-scale preparation of PLA films with mechanical robustness and superhydrophobicity and could broaden their application scope to self-cleaning and moisture-proof fields." @default.
- W4380489021 created "2023-06-14" @default.
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- W4380489021 date "2023-06-13" @default.
- W4380489021 modified "2023-10-17" @default.
- W4380489021 title "Polylactide Films with Superhydrophobicity and Superior Mechanical Properties Constructed by Combining Annealing Stretching and Nonsolvent-Induced Phase Separation" @default.
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- W4380489021 doi "https://doi.org/10.1021/acssuschemeng.3c01938" @default.
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