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- W4380729958 abstract "We have developed a one-pot synthetic method for producing 1,2-diamines from easily prepared and commercially available precursors through a formal umpolung process. Our method utilizes an efficient [3 + 2] cycloaddition as the key step in forming substituted 1,2-diamines in moderate to high yields. These resulting compounds can undergo subsequent transformations, demonstrating their utility as synthetic building blocks for more complex scaffolds. Finally, we propose a reasonable mechanism for this transformation using density functional theory modeling, justifying the experimental observations." @default.
- W4380729958 created "2023-06-16" @default.
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- W4380729958 date "2023-06-15" @default.
- W4380729958 modified "2023-10-15" @default.
- W4380729958 title "[3 + 2] Cycloadditions of Tertiary Amine <i>N</i>-Oxides and Silyl Imines as an Innovative Route to 1,2-Diamines" @default.
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- W4380729958 doi "https://doi.org/10.1021/acs.orglett.3c01396" @default.
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