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- W4380994078 abstract "Strong light-matter coupling provides a versatile and novel means to manipulate chemical processes. Here we develop a theoretical framework to investigate the spectroscopy and dynamics of a molecular ensemble embedded in an optical cavity under the collective strong coupling regime. This theory is constructed by a pseudoparticle representation of the molecular Hamiltonians, mapping the polaritonic Hamiltonian into a coupled fermion-boson model under particle number constraints. The mapped model is then analyzed using the non-equilibrium Green function theory with the important self-energy diagrams identified through power counting. Numerical demonstrations are shown for the driven Tavis-Cummings model, which shows an excellent agreement with exact results." @default.
- W4380994078 created "2023-06-17" @default.
- W4380994078 creator A5091667861 @default.
- W4380994078 date "2023-06-15" @default.
- W4380994078 modified "2023-09-26" @default.
- W4380994078 title "Toward collective chemistry by strong light-matter coupling" @default.
- W4380994078 doi "https://doi.org/10.48550/arxiv.2306.08944" @default.
- W4380994078 hasPublicationYear "2023" @default.
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