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- W4381056800 abstract "In this study, we design a triphasic Ni2P−Fe2P−CoP heterostructure appearing under the form of a hierarchical 3D core–shell hybrid ([email protected]2P−Fe2P) for bifunctionally catalyzing both hydrogen evolution reaction (HER) and oxygen evolution reaction (OER) in alkaline medium. Density functional theory results indicate that the rich interfaces of Ni2P−Fe2P−CoP architecture exhibit the best electronic properties and enhanced multiple electroactive site number with optimum hydrogen adsorption energy, significantly surpassing the CoP, CoP−Ni2P, or CoP−Fe2P cases. Therefore, the electrolyzer cell of [email protected]2P−Fe2P(+,−) requires a small operating voltage of 1.51 V to reach 10 mA cm−2 during alkaline water splitting, outperforming the commercial catalyst couple of Pt/C(–)//RuO2(+) and numerous earlier reports. In addition, the solar-driven water splitting system demonstrates a high solar-to-hydrogen (STH) conversion of 15.33%, along with excellent long-term stability. The results open a potential approach to design innovative high-performance electrocatalysts for practical green hydrogen production via electrochemical water splitting process." @default.
- W4381056800 created "2023-06-18" @default.
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- W4381056800 date "2023-12-01" @default.
- W4381056800 modified "2023-10-05" @default.
- W4381056800 title "Triphasic Ni2P−Fe2P−CoP Heterostructure Interfaces for Efficient Overall Water Splitting Powered by Solar Energy" @default.
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- W4381056800 doi "https://doi.org/10.1016/j.apcatb.2023.123016" @default.
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