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- W4381186875 abstract "MIL-100(Fe) is a kind of metal-organic frameworks (MOFs) with robust water and chemical stability. The adsorption kinetics, isotherms, thermodynamics and regeneration of MIL-100(Fe) were investigated to illustrate the process of efficient lithium adsorption. The adsorption kinetics of MIL-100(Fe) followed Pseudo-second-order model, and the lithium adsorption equilibrium was reached rapidly in 2 h. Langmuir model fit best with the adsorption isotherms, indicating chemisorption of lithium ions on MIL-100(Fe) and possibly a monolayer adsorption process. By calculating thermodynamic parameters (ΔGθ, ΔHθ and ΔS θ), the adsorption of lithium on MIL-100(Fe) can be illustrated by a spontaneous endothermic process. The adsorption mechanism involved electrostatic interaction, impact of crystal defect sites and coordinative interactions between metal active sites and lithium ions (Fe—F‧‧‧Li). MIL-100(Fe) was regenerated for four cycles, and there was only a slightly decrease in adsorption capacity and the morphology remained stable. Combined with extremely short equilibrium time and high stability, MIL-100(Fe) can be a promising adsorbent for lithium extraction." @default.
- W4381186875 created "2023-06-20" @default.
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- W4381186875 date "2023-10-01" @default.
- W4381186875 modified "2023-10-15" @default.
- W4381186875 title "Efficient lithium extraction from aqueous solutions by MIL-100(Fe): A study on adsorption kinetics, thermodynamics and mechanism" @default.
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- W4381186875 doi "https://doi.org/10.1016/j.seppur.2023.124365" @default.
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