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- W4381194951 abstract "Photoexcited charge separation and their efficient transportation in bulk as well as in heterojunction based photocatalysts is a challenging issue. Therefore, seeding free BiVO4@Fe-TiO2 NRs heterojunction is developed to have molecular extrinsic defects via Fe doping in TiO2 nanorods (NRs) as a strategy in type-II heterojunctions for photoelectrochemical water splitting. Structural characterizations of BiVO4@Fe-TiO2 NRs confirm the introduction of extrinsic defects in doped Fe-TiO2 NRs. Morphological studies evaluate the homogeneous deposition of BiVO4@Fe-TiO2 NRs to form core-shell heterostructure. In photoelectrochemical studies, BiVO4@0.2%Fe-TiO2 shows highest photocurrent density of 1.52mA/cm2 in comparison to BiVO4@undoped TiO2 NRs with 0.52mA/cm2 and pristine TiO2 NRs with 45μA/cm2 at 1.23 vs. RHE under 100mW/cm2 light intensity. These findings elucidate the importance of modified host substrates of Fe-TiO2 NRs to extract photoexcited electrons from guest BiVO4 that has enhanced PEC performance with maximum electron mobility, efficient interfacial charge transfer and enhanced electron quenching window in type-II heterojunctions." @default.
- W4381194951 created "2023-06-20" @default.
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- W4381194951 date "2023-10-01" @default.
- W4381194951 modified "2023-09-26" @default.
- W4381194951 title "Boosting the Photoexcited Charge Collection and Transportation via BiVO4/Fe-TiO2 NRs in Type-II Heterojunction for Efficient Photoelectrochemical Water Splitting" @default.
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- W4381194951 doi "https://doi.org/10.1016/j.jphotochem.2023.114956" @default.
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