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- W4381381672 abstract "To enhance photoelectrochemical (PEC) performance, additional electron donor/acceptor is generally required to inhibit the electron-hole recombination. However, the enhancement is limited due to the long-distance diffusion. Herein a self-supplying electron strategy is designed for PEC enhancement by coordinating an electron donor 1.4-diazabicyclo[2.2.2]octane (Dabco) in metal–organic framework (MOF). The intrareticular photoelectron transfer mechanism in mixed-ligand MOF (m-MOF) is experimentally revealed and verified by density functional theory calculations. The presence of Dabco efficiently inhibits the electron-hole recombination due to the self-supplying electrons and longer electron lifetime in the framework, and thus leads to 23.2-fold enhancement of photocurrent. As proof of concept, a simple PEC method is constructed with the designed m-MOF to demonstrate its application in sensitive bioanalysis. This work provides a new avenue for improving the PEC performance of nanomaterials." @default.
- W4381381672 created "2023-06-21" @default.
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- W4381381672 date "2023-07-04" @default.
- W4381381672 modified "2023-10-14" @default.
- W4381381672 title "Electron Donor Coordinated Metal‐Organic Framework to Enhance Photoelectrochemical Performance" @default.
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- W4381381672 doi "https://doi.org/10.1002/ange.202308514" @default.
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