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- W4381470188 abstract "Reported herein is the catalytic asymmetric aminative dearomatization reaction of common phenols. As opposed to the well-studied indoles and naphthols, phenols are supposed to be challenging substrates for catalytic asymmetric dearomatization reactions in terms of their strong aromaticity and regioselectivity issues. Under the catalysis of a chiral phosphoric acid, the C4-regiospecific aminative dearomatization of phenols with azodicarboxylates readily occurred at ambient temperature, delivering an array of biologically and synthetically important aza-quaternary carbon cyclohexadieneones in good yields and with excellent enantioselectivities (29 examples, up to 98% yield, and >99% ee)." @default.
- W4381470188 created "2023-06-22" @default.
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- W4381470188 date "2023-06-21" @default.
- W4381470188 modified "2023-10-16" @default.
- W4381470188 title "Catalytic Asymmetric Synthesis of Aza-Quaternary Carbon Cyclohexadieneones Enabled by Aminative Dearomatization of Phenols" @default.
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- W4381470188 doi "https://doi.org/10.1021/acs.orglett.3c01746" @default.
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