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- W4381470233 abstract "The coordination structure determines the electrocatalytic performances of single atom catalysts (SACs), while it remains a challenge to precisely regulate their spatial location and coordination environment. Herein, we report a universal sub-nanoreactor strategy for synthesis of yolk–shell MoS2 supported single atom electrocatalysts with dual–anchored microenvironment of vacancy-enriched MoS2 and intercalation carbon toward robust hydrogen-evolution reaction. Theoretical calculations reveal that the “E-Lock” and “E-Channel” are conducive to stabilize and activate metal single atoms. A group of SACs is subsequently produced with the assistance of sulfur vacancy and intercalation carbon in the yolk–shell sub-nanoreactor. The optimized C-Co-MoS2 yields the lowest overpotential (η10=17 mV) compared with previously reported MoS2-based electrocatalysts to date, and also affords a 5‒9 fold improvement in activity even comparing with those as-prepared single–anchored analogues. Theoretical results and in-situ characterizations unveil its active center and durability. This work provides a universal pathway to design efficient catalysts for electro-refinery." @default.
- W4381470233 created "2023-06-22" @default.
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- W4381470233 date "2023-06-21" @default.
- W4381470233 modified "2023-10-14" @default.
- W4381470233 title "Universal Sub‐Nanoreactor Strategy for Synthesis of Yolk‐Shell MoS2 Supported Single Atom Electrocatalysts toward Robust Hydrogen Evolution Reaction" @default.
- W4381470233 doi "https://doi.org/10.1002/anie.202308091" @default.
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