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• W4381487430 abstract "The p-i heterojunction imbedded underneath the perovskite layer plays a vital role in determining the efficiency and stability of inverted perovskite solar cells (PSCs). We found that poly[bis(4-phenyl) (2,4,6-trimethylphenyl) amine] (PTAA) suffers from the severely chain entanglement resulting in poor contact with perovskite. In this work, PTAA layer was treated by poly[(2,6-(4,8-bis(5-(2-ethylhexylthio)-4-fluorothiophen-2-yl)-benzo[1,2-b:4,5-b′] dithiophene))-alt-(5,5-(1′,3′-di-2-thienyl-5′,7′-bis(2-ethylhexyl) benzo[1′,2′-c:4′,5′-c′] dithiophene-4,8-dione)] (PBDB-T-SF) diluted solution in chlorobenzene. PBDB-T-SF, which contains dual carbonyl groups in its backbones and suitable electronic levels, can spontaneously fill the voids in chlorobenzene-washed PTAA (nano-PTAA). This not only promotes the work function of the substrate but also strengthens the coherence between perovskite and the substrate. Blade coated PSC (0.09 cm2) containing PBDB-T-SF (s-PSCs) realized a power conversion efficiency (PCE) of 21.83 %. After aging for more than 2000 hours, s-PSCs maintains 88 % of the initial efficiency which is only 59 % for the control devices." @default.
• W4381487430 created "2023-06-22" @default.
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• W4381487430 date "2023-06-01" @default.
• W4381487430 modified "2023-09-24" @default.
• W4381487430 title "Heteropolymer improves p-i junction in perovskite solar cells" @default.
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• W4381487430 doi "https://doi.org/10.1016/j.jcis.2023.06.070" @default.
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