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- W4381716405 abstract "Abstract Lithium difluoro(oxalato) borate (LiDFOB) has been widely investigated in lithium‐ion batteries (LIBs) owing to its advantageous thermal stability and excellent aluminum passivation property. However, LiDFOB tends to suffer from severe decomposition and generate a lot of gas species (e.g., CO 2 ). Herein, a novel cyano‐functionalized lithium borate salt, namely lithium difluoro(1,2‐dihydroxyethane‐1,1,2,2‐tetracarbonitrile) borate (LiDFTCB), is innovatively synthesized as a highly oxidative‐resistant salt to alleviate above dilemma. It is revealed that the LiDFTCB‐based electrolyte enables LiCoO 2 /graphite cells with superior capacity retention at both room and elevated temperatures (e.g., 80 % after 600 cycles) with barely any CO 2 gas evolution. Systematic studies reveal that LiDFTCB tends to form thin and robust interfacial layers at both electrodes. This work emphasizes the crucial role of cyano‐functionalized anions in improving cycle lifespan and safety of practical LIBs." @default.
- W4381716405 created "2023-06-24" @default.
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- W4381716405 date "2023-07-13" @default.
- W4381716405 modified "2023-10-17" @default.
- W4381716405 title "Highly Oxidative‐Resistant Cyano‐Functionalized Lithium Borate Salt for Enhanced Cycling Performance of Practical Lithium‐Ion Batteries" @default.
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- W4381716405 doi "https://doi.org/10.1002/anie.202302664" @default.
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