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• W4381853744 abstract "We report the experimental observation of quantum interference in the nuclear wave-packet dynamics driving ultrafast excitation-energy transfer in argon dimers below the threshold of interatomic Coulombic decay (ICD). Using time-resolved photoion-photoion coincidence spectroscopy and quantum dynamics simulations, we reveal that the electronic relaxation dynamics of the inner-valence 3s hole on one atom leading to a 4s or 4p excitation on the other one is influenced by nuclear quantum dynamics in the initial state, giving rise to a deep, periodic modulation on the kinetic-energy-release (KER) spectra of the coincident Ar^{+}-Ar^{+} ion pairs. Moreover, the time-resolved KER spectra show characteristic fingerprints of quantum interference effects during the energy-transfer process. Our findings pave the way to elucidating quantum-interference effects in ultrafast charge- and energy-transfer dynamics in more complex systems, such as molecular clusters and solvated molecules." @default.
• W4381853744 created "2023-06-25" @default.
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• W4381853744 date "2023-06-23" @default.
• W4381853744 modified "2023-10-13" @default.
• W4381853744 title "Observation of Nuclear Wave-Packet Interference in Ultrafast Interatomic Energy Transfer" @default.
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• W4381853744 doi "https://doi.org/10.1103/physrevlett.130.253202" @default.
• W4381853744 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/37418708" @default.
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