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- W4381887746 abstract "Abstract The zero‐length column (ZLC) method has been frequently used to measure the effective diffusivity of guest molecules in nanoporous crystalline materials. Recent studies unveiled that the mass transport of guest molecules could originate from either intracrystalline diffusion and/or surface barriers. Directly quantifying the intracrystalline diffusivity and surface permeability of guest molecules. therefore, is essential for understanding the mass transfer and thus optimizing the design of nanoporous crystalline materials. In this work, we extended the ZLC method, based on a derived theoretical expression of the desorption rate, to decouple the surface barriers and intracrystalline diffusion from effective diffusion of guest molecules in nanoporous materials. The diffusivities of ethane, propane and n‐pentane in SAPO‐34 and Beta zeolites have been experimentally measured to verify the effectiveness of this method." @default.
- W4381887746 created "2023-06-25" @default.
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- W4381887746 date "2023-06-21" @default.
- W4381887746 modified "2023-10-14" @default.
- W4381887746 title "Quantifying molecular surface barriers and intracrystalline diffusion in nanoporous materials by zero‐length column" @default.
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- W4381887746 doi "https://doi.org/10.1002/aic.18159" @default.
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