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• W4382010269 abstract "Most of previous studies proved bicarbonate (HCO₃^-) was free radical scavenger in advanced oxidation processes, however, in this study, the positive influence of HCO₃^- was confirmed in heterogeneous Fenton. The results showed that the degradation efficiency of Rhodamine B increased from 13.7% to 95.3% by adding appropriate concentration of HCO₃^-, and the zeolite supported Co and Cu oxides (Co/Cu/zeolite) could catalyze the HCO₃^- enhanced Fenton process. The response surface method was employed to optimize the concentration of HCO₃^- needed in the heterogeneous Fenton system. Radicals quenching results showed that ¹O₂ and O₂^·- rather than ·OH played important roles in the degradation of Rhodamine B. Mechanism studies indicated that carbonate radical (CO₃^·-) was the key intermediate in the formation of ¹O₂ and O₂^·-, and CO₃^·- could be generated through the reaction between HCO₃^- and ·OH. In addition, peroxymonocarbonate (HCO₄^-), which further produced CO₃^·-, was also generated in the bicarbonate enhancement system. The electron transfer between Cu and Co promoted the heterogeneous Fenton process in generating ·OH that reacted with HCO₃^-, or catalyzed HCO₄^- to generate CO₃^·-." @default.
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• W4382010269 date "2023-04-24" @default.
• W4382010269 modified "2023-10-01" @default.
• W4382010269 title "Insights into bicarbonate enhanced heterogeneous Fenton catalyzed by Co/Cu/zeolite for degradation of rhodamine B" @default.
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• W4382010269 doi "https://doi.org/10.4491/eer.2023.095" @default.
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