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- W4382020723 abstract "Abstract Achieving high solar-to-hydrogen (STH) efficiency concomitant with long-term durability using low-cost, scalable photo-absorbers is a long-standing challenge. Here we report the design and fabrication of a conductive adhesive-barrier (CAB) that translates >99% of photoelectric power to chemical reactions. The CAB enables halide perovskite-based photoelectrochemical cells with two different architectures that exhibit record STH efficiencies. The first, a co-planar photocathode-photoanode architecture, achieved an STH efficiency of 13.4% and 16.3 h to t 60 , solely limited by the hygroscopic hole transport layer in the n-i-p device. The second was formed using a monolithic stacked silicon-perovskite tandem, with a peak STH efficiency of 20.8% and 102 h of continuous operation before t 60 under AM 1.5G illumination. These advances will lead to efficient, durable, and low-cost solar-driven water-splitting technology with multifunctional barriers." @default.
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- W4382020723 date "2023-06-26" @default.
- W4382020723 modified "2023-10-18" @default.
- W4382020723 title "Integrated halide perovskite photoelectrochemical cells with solar-driven water-splitting efficiency of 20.8%" @default.
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- W4382020723 doi "https://doi.org/10.1038/s41467-023-39290-y" @default.
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