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W4382048105 abstract "Constructing Van der Waals heterojunction is a crucial strategy to achieve excellent photocatalytic activity. However, in most Van der Waals heterojunctions synthesized by ex situ assembly, electron transfer encounters huge hindrances at the interface between the two components due to the large spacing and potential barrier. Herein, a phosphate-bridged Van der Waals heterojunction of cobalt phthalocyanine (CoPc)/tungsten disulfide (WS2 ) bridged by phosphate (xCoPc-nPO4- -WS2 ) is designed and prepared by the traditional wet chemistry method. By introducing a small phosphate molecule into the interface of CoPc and WS2 , creates an electron bridge, resulting in a compact combination and eliminating the space barrier. Therefore, the phosphate (PO4- ) bridge can serve as an efficient electron transfer channel in heterojunction and can efficiently transmit photoelectrons from WS2 to CoPc under excited states. These excited photoelectrons are captured by the catalytic central Co2+ in CoPc and subsequently convert CO2 molecules into CO and CH4 products, achieving 17-fold enhancement on the 3CoPc-0.6PO4- -WS2 sample compared to that of pure WS2 . Introducing a small molecule bridge to create an electron transfer channel provides a new perspective in designing efficient photocatalysts for photocatalytic CO2 reduction into valuable products." @default.
W4382048105 created "2023-06-27" @default.
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W4382048105 date "2023-07-30" @default.
W4382048105 modified "2023-10-16" @default.
W4382048105 title "Photoelectron “Bridge” in Van Der Waals Heterojunction for Enhanced Photocatalytic CO<sub>2</sub> Conversion Under Visible Light" @default.
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W4382048105 doi "https://doi.org/10.1002/adma.202303047" @default.
W4382048105 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/37363951" @default.
W4382048105 hasPublicationYear "2023" @default.
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