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- W4382051323 endingPage "144415" @default.
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- W4382051323 abstract "Core-shell structured explosives (CSEs) are becoming increasingly prominent in the energetic materials, however, some fatal defects of CSEs including inadequate two-phase adhesion, insufficient shell coverage and thickness, and poor chemical stability seriously impact the security and dependability of weapon systems. Herein, we present a novel core-shell material in the field of organic crystals, the core@self-shell structure, constructed by an original strategy of autologous surface molecular reconfiguration. The solvate dioxane (DIOX) of 4,4′,5,5′-tetranitro-1H,1′H-[2,2′-biimidazole]-1,1′-diamine (DATNBI) that screening based on computational prediction has the propensity to form a unique nanostructure after drying. According to this finding, we successfully designed the core@self-shell structure with a hierarchical nano-surface and proposed the “solvate micro-dissolution shell” formation mechanism. The core@self-shell energetic nanomaterials significantly improve impact sensitivity (22.5 J, raw material: 12 J) without greatly decreasing energy density through the eco-friendly and effective method, presenting great potential for industrial applications due to its excellent performance and simple construction process." @default.
- W4382051323 created "2023-06-27" @default.
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- W4382051323 date "2023-09-01" @default.
- W4382051323 modified "2023-09-27" @default.
- W4382051323 title "Constructing core@self-shell structured energetic nanomaterials by autologous surface molecular reconfiguration: The DATNBI case" @default.
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- W4382051323 doi "https://doi.org/10.1016/j.cej.2023.144415" @default.
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