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- W4382073723 abstract "The increasing demand for lithium and limited resources has attracted attention to challenging omnipresent resources like seawater, where the commonly used Li2CO3 precipitation method fails. Lithium-selective receptors could, in principle, circumvent these challenges but are plagued by poor extraction ability from dilute solutions. In this work, we report new anthraquinone-derived acyclic ionophores that undergo self-assembly to form a very stable binuclear lithium adduct, selective over sodium & potassium analogs, supported by DFT studies and crystal structures. Consequently, a high binding constant (Ka ∼ 105 M−1) and lithium recognition at a nanomolar concentration (LOD ∼ 90 nM) were observed. The high binding affinity and stability of lithium adduct efficiently drive lithium-ions transportation and solvent extraction from dilute solutions with a lithium concentration as low as 10 ppm and from sea bittern. This study opens an avenue to circumvent the limitations for future lithium sequestration even from natural resources." @default.
- W4382073723 created "2023-06-27" @default.
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- W4382073723 date "2023-08-01" @default.
- W4382073723 modified "2023-10-15" @default.
- W4382073723 title "Lithium sequestration from dilute solutions and sea bittern inspired by the self-assembled complexation" @default.
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- W4382073723 doi "https://doi.org/10.1016/j.cej.2023.144408" @default.
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